Spin texture induced by non-magnetic doping and spin dynamics in 2D triangular lattice antiferromagnet <i> h </i> -Y(Mn,Al)O 3

Abstract

'Jonathan C. Leiner' 'Hasung Sim' 'Taehun Kim' 'Jaehong Jeong' 'Kirrily C. Rule' 'Kazuya Kamazawa' 'Kazuki Iida' 'T. G. Perring' 'Hyungje Woo' 'S.-W. Cheong' 'M. E. Zhitomirsky' 'A. L. Chernyshev' 'Je-Geun Park'] Novel effects induced by nonmagnetic impurities in frustrated magnets and quantum spin liquid represent a highly nontrivial and interesting problem. A theoretical proposal of extended modulated spin structures induced by doping of such magnets, distinct from the well-known skyrmions has attracted significant interest. Here, we demonstrate that nonmagnetic impurities can produce such extended spin structures in h-YMnO3, a triangular antiferromagnet with noncollinear magnetic order. Using inelastic neutron scattering (INS), we measured the full dynamical structure factor in Al-doped h-YMnO3 and confirmed the presence of magnon damping with a clear momentum dependence. Our theoretical calculations can reproduce the key features of the INS data, supporting the formation of the proposed spin textures. As such, our study provides the first experimental confirmation of the impurity-induced spin textures. It offers new insights and understanding of the impurity effects in a broad class of noncollinear magnetic systems.